Compositions and sources of sedimentary organic carbon on the tropical epicontinental sea
编号:2921
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更新:2023-04-12 18:58:18 浏览:531次
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摘要
The deposition of fluvially derived terrestrial organic carbon (OC) together with marine OC in marine sediments has important implications for the global carbon cycle. However, dispersal extent and fates of terrestrial soil and petrogenic OC on the continental shelf have remained unclear and debated. Here, we present OC compositions and mineral properties of marine sediments from the Gulf of Thailand and the adjacent Mekong shelf, as well as river sediments from continents surrounding them in order to determine the provenance of sedimentary OC in this tropical epicontinental sea. We find that stable carbon isotope composition (δ13C) and radiocarbon activity (Δ14C) of sedimentary OC fall between those of marine OC and of river sediments, mainly composed of C3 plant-dominated pre-aged soil and petrogenic OC. Mixing model reveals that the OC in river sediments is predominantly sourced from pre-aged deep soils, accounting for 70 ± 6%, with the remaining consisting of modern surface soil (23 ± 5%), riverine primary productivity (4 ± 2%), and bedrock (2 ± 1%). The sedimentary OC on the shelf is primarily derived from marine OC, accounting for 65 ± 15%, with terrestrial soil OC and petrogenic OC contributing 24 ± 14% and 10 ± 5%, respectively. The sources, degradation, and aging of OC and mineral surface area determine the spatial pattern of sedimentary OC compositions in the Gulf of Thailand and the Mekong shelf. The contents of marine, soil, and petrogenic OC decrease with increasing distance offshore, consistent with changes in spatial patterns of sedimentation rate of terrestrial materials and of marine primary production in the overlying water column. Extensive degradation of terrestrial OC and extremely low OC burial rate in this tropical epicontinental sea suggest a minor role on OC sequestration in marine sediments in the context of the global carbon cycle.
关键词
Radiocarbon, Organic carbon, River sediments, Marine sediments, Tropical epicontinental sea
稿件作者
林宝治
同济大学
刘志飞
同济大学
赵美训
中国海洋大学
SompongchaiyakulPenjai
Chulalongkorn University
张海龙
中国海洋大学
BlattmannThomas M.
ETH Zürich
冯铄
同济大学
WiesnerMartin G.
自然资源部第二海洋研究所,卫星海洋环境动力学国家重点实验室
LeKhanh Phon
Hanoi University of Mining and Geology
MeasRithy
Department of Coastal Zone and Marine Conservation, Ministry of Environment
SathiamurthyEdlic
University Malaysia Terengganu
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